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4 8 , 3 419. 61. N. ( 1 9 8 2 ) . Adv. , 1J5, 3 1 ; Klein, J. ( 1 9 8 2 ) . Adv. , 1 6 , 101. E. H. P. V. G. H. E. T. Podoll C. F. Billett R. E. W. J. Greenleaf P. G. J. J. Szanto J. P. Fletcher C. Foster THERMODYNAMICS OF ADSORPTION FROM MIXED SOLVENTS Denver G. Hall Unilever Research Port Sunlight Laboratory Quarry Road East, Behington, Wirral, Merseyside L63 3JW ABSTRACT A general thermodynamic treatment of adsorption from mixed solvents is provided. It is designed to apply in situations where adsorbed species may be regarded as distinct from their bulk counterparts.

1 p. - I V (26) c where v denotes ionic valence and includes the sign and where species c is chosen for convenience but is otherwise arbitrary. The 0-j_ play the same role as the chemical potentials of uncharged species and when they are included in the above formalism where appropriate no further modi­ fications are required. (3) Some of the derivatives in equations 12 and 25 require more variables to be held constant than is possible at equilibrium. To use these expressions when only equilibrium data are available it may be necessary to estimate these derivatives by arguing that some are negligible and that the others can be approximated by quantities which are obtainable solely from equilibrium data.

Faraday Soc, 40, 177. 20. H. H. (1968), Trans. Faraday Soc, _64, 2639. 21. Bown, R, (1973). D. Thesis, Bristol. 22. , (1978). Progr. , 65, 103. 23. H. J. (1964). , 60, 1951. 24. I. (1967). "Phase Equilibrium and Surface Phenomena", Chapter VI, Chimia, Leningrad. 25. H. J. (1975). S. Faraday I, 71, 883. 26. Defay, R. and Prigogine, I. (1950). Faraday Soc, 46, 199. 27. Ono, S. (1947). , Tamura, M, and Kurata, M. (1951). Phys. Soc. Japan, 6>, 309; Ono, S. and Kondo S. (1960). I n "Encyclopaedia of Physics" (ed.

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